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Abstract A new method that automatically determines the modality of an observed particle size distribution (PSD) and the representation of each mode as a gamma function was used to characterize data obtained during the High Altitude Ice Crystals and High Ice Water Content (HAIC-HIWC) project based out of Cayenne, French Guiana, in 2015. PSDs measured by a 2D stereo probe and a precipitation imaging probe for particles with maximum dimension ( D max ) > 55 μ m were used to show how the gamma parameters varied with environmental conditions, including temperature ( T ) and convective properties such as cloud type, mesoscale convective system (MCS) age, distance away from the nearest convective peak, and underlying surface characteristics. Four kinds of modality PSDs were observed: unimodal PSDs and three types of multimodal PSDs (Bimodal1 with breakpoints 100 ± 20 μ m between modes, Bimodal2 with breakpoints 1000 ± 300 μ m, and Trimodal PSDs with two breakpoints). The T and ice water content (IWC) are the most important factors influencing the modality of PSDs, with the frequency of multimodal PSDs increasing with increasing T and IWC. An ellipsoid of equally plausible solutions in ( N o – λ–μ ) phase space is defined for each mode of the observed PSDs for different environmental conditions. The percentage overlap between ellipsoids was used to quantify the differences between overlapping ellipsoids for varying conditions. The volumes of the ellipsoid decrease with increasing IWC for most cases, and ( N o – λ–μ ) vary with environmental conditions related to distribution of IWC. HIWC regions are dominated by small irregular ice crystals and columns. The parameters ( N o – λ–μ ) in each mode exhibit mutual dependence. 

Abstract High Ice Water Content (HIWC) regions above tropical mesoscale convective systems are investigated using data from the second collaboration of the High Altitude Ice Crystals and High Ice Water Content projects (HAIC-HIWC) based in Cayenne, French Guiana in 2015. Observations from in-situ cloud probes on the French Falcon 20 determine the microphysical and thermodynamic properties of such regions. Data from a 2-D stereo probe and precipitation imaging probe show how statistical distributions of ice crystal mass median diameter ( MMD ), ice water content ( IWC ), and total number concentration ( N t ) for particles with maximum dimension ( D max ) > 55 μm vary with environmental conditions, temperature ( T ), and convective properties such as vertical velocity ( w ), MCS age, distance away from convective peak ( L ), and surface characteristics. IWC is significantly correlated with w , whereas MMD decreases and N t increases with decreasing T consistent with aggregation, sedimentation and vapor deposition processes at lower altitudes. MMD typically increases with IWC when IWC < 0.5 g m -3 , but decreases with IWC when IWC > 0.5 g m -3 for -15 °C ≤ T ≤ -5 °C. Trends also depend on environmental conditions, such as presence of convective updrafts that are the ice crystal source, MMD being larger in older MCSs consistent with aggregation and less injection of small crystals into anvils, and IWC s decrease with increasing L at lower T . The relationship between IWC and MMD depends on environmental conditions, with correlations decreasing with decreasing T . The strength of correlation between IWC and N t increases as T decreases. 

Microorganisms are ubiquitous and highly diverse in the atmosphere. Despite the potential impacts of airborne bacteria found in the lower atmosphere over the Southern Ocean (SO) on the ecology of Antarctica and on marine cloud phase, no previous region-wide assessment of bioaerosols over the SO has been reported. We conducted bacterial profiling of boundary layer shipboard aerosol samples obtained during an Austral summer research voyage, spanning 42.8 to 66.5°S. Contrary to findings over global subtropical regions and the Northern Hemisphere, where transport of microorganisms from continents often controls airborne communities, the great majority of the bacteria detected in our samples were marine, based on taxonomy, back trajectories, and source tracking analysis. Further, the beta diversity of airborne bacterial communities varied with latitude and temperature, but not with other meteorological variables. Limited meridional airborne transport restricts southward community dispersal, isolating Antarctica and inhibiting microorganism and nutrient deposition from lower latitudes to these same regions. A consequence and implication for this region’s marine boundary layer and the clouds that overtop it is that it is truly pristine, free from continental and anthropogenic influences, with the ocean as the dominant source controlling low-level concentrations of cloud condensation nuclei and ice nucleating particles. 

This study focuses on methods to estimate dry marine aerosol surface area (SA) from bulk optical measurements. Aerosol SA is used in many models' ice nucleating particle (INP) parameterizations, as well as influencing particle light scattering, hygroscopic growth, and reactivity, but direct observations are scarce in the Southern Ocean (SO). Two campaigns jointly conducted in austral summer 2018 provided co‐located measurements of aerosol SA from particle size distributions and lidar to evaluate SA estimation methods in this region. Mie theory calculations based on measured size distributions were used to test a proposed approximation for dry aerosol SA, which relies on estimating effective scattering efficiency (Q) as a function of Ångström exponent (å). For distributions with dryå< 1,Q = 2 was found to be a good approximation within ±50%, but for distributions with dryå> 1, an assumption ofQ = 3 as in some prior studies underestimates dry aerosol SA by a factor of 2 or more. We propose a new relationship between dryåandQ, which can be used for −0.2 <å< 2, and suggestå = 0.8 as the cutoff between primary and secondary marine aerosol‐dominated distributions. Application of a published methodology to retrieve dry marine aerosol SA from lidar extinction profiles overestimated aerosol SA by a factor of 3–5 during these campaigns. Using Microtops aerosol optical thickness measurements, we derive alternative lidar conversion parameters from our observations, applicable to marine aerosol over the SO.

 

Abstract Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation and radiative processes, and their interactions. Projects between 2016 and 2018 used in-situ probes, radar, lidar and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN) and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase cloudsnucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF/NCAR G-V aircraft flying north-south gradients south of Tasmania, at Macquarie Island, and on the RV Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show a largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multi-layered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of confirmed low clouds were responsible for radiation biases. The combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets.